Charge distribution induced inside complex plasmonic nanoparticles.

نویسندگان

  • R Marty
  • G Baffou
  • A Arbouet
  • C Girard
  • R Quidant
چکیده

We developed a versatile numerical technique to compute the three-dimensional charge distribution inside plasmonic nanoparticles. This method can be easily applied to investigate the charge distribution inside arbitrarily complex plasmonic nanostructures and to identify the nature of the multipolar plasmon modes involved at plasmonic resonances. Its ability to unravel the physical origin of plasmonic spectral features is demonstrated in the case of a single gold nanotriangle and of a gold nano-antenna. Finally, we show how the volume charge distribution can be used to define and compute the first terms of the multipolar expansion.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Simulation of Surface Plasmon Excitation in a Plasmonic Nano-Wire Using Surface Integral Equations

In this paper, scattering of a plane and monochromatic electromagnetic wave from a nano-wire is simulated using surface integral equations. First, integral equationsgoverning unknown fields on the surface is obtained based on Stratton-Cho surface integral equations. Then, the interaction of the wave with a non-plasmonic as well as a palsmonic nano-wire is considered. It is shown that in scatter...

متن کامل

Evidence and implications of direct charge excitation as the dominant mechanism in plasmon-mediated photocatalysis

Plasmonic metal nanoparticles enhance chemical reactions on their surface when illuminated with light of particular frequencies. It has been shown that these processes are driven by excitation of localized surface plasmon resonance (LSPR). The interaction of LSPR with adsorbate orbitals can lead to the injection of energized charge carriers into the adsorbate, which can result in chemical trans...

متن کامل

The UV Plasmonic Behavior of Distorted Rhodium Nanocubes

For applications of surface-enhanced spectroscopy and photocatalysis, the ultraviolet (UV) plasmonic behavior and charge distribution within rhodium nanocubes is explored by a detailed numerical analysis. The strongest plasmonic hot-spots and charge concentrations are located at the corners and edges of the nanocubes, exactly where they are the most spectroscopically and catalytically active. B...

متن کامل

Nanoscale control of optical heating in complex plasmonic systems.

We introduce a numerical technique to investigate the temperature distribution in arbitrarily complex plasmonic systems subject to external illumination. We perform both electromagnetic and thermodynamic calculations based upon a time-efficient boundary element method. Two kinds of plasmonic systems are investigated in order to illustrate the potential of such a technique. First, we focus on in...

متن کامل

Plasmonic ELISA for the ultrasensitive detection of Treponema pallidum.

In this report, we have developed a plasmonic ELISA strategy for the detection of syphilis. Plasmonic ELISA is an enzyme-linked immunoassay combined with enzyme-mediated surface plasmon resonance (SPR) of gold nanoparticles (AuNPs). Immune response of the Treponema pallidum (T. pallidum) antibodies triggers the acetylcholinesterase-catalyzed hydrolysis of acetylthiocholine to produce abundant t...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Optics express

دوره 18 3  شماره 

صفحات  -

تاریخ انتشار 2010